中文版 | English
Title

Experimental study of the influence of geochemical features on the viscoelasticity of organic matter in shale

Author
Corresponding AuthorZhang, Dongxiao
Publication Years
2022-09-01
DOI
Source Title
ISSN
0264-8172
EISSN
1873-4073
Volume143
Abstract
Understanding time-dependent mechanical properties is critical to perform geomechanical risk quantification and reduce the environmental impact of fracking operations. In this study, vitrinite reflectance test, scanning electron microscope (SEM)/helium ion microscope (HIM) observation, atomic force microscopy (AFM)-based nanoscale dynamic mechanical analysis (AFM-nDMA), and micro-Raman analysis were combined as a chemomechanical method to investigate the role of thermal maturation in affecting nanoscale viscoelasticity of organic matter with maceral classification. The results of 208 tested areas demonstrated that viscosity is negatively correlated with thermal maturity, while storage modulus is positively correlated with maturity, suggesting that such polymer-like to mineral-like process might be prone to fracture initiation. Moreover, chemical structure changes during the thermal evolution exhibited by micro-Raman analysis were found to contribute to the abovementioned mechanical variations. Characterization of viscoelasticity of organic matter considering geochemical features is a highly promising aspect for inclusion in petrophysical workflows, leading to improved design of hydraulic fracturing and homogenization modeling.
Keywords
URL[Source Record]
Indexed By
SCI ; EI
Language
English
SUSTech Authorship
Corresponding
Funding Project
Shenzhen Key Laboratory of Natural Gas Hydrates[ZDSYS20200421111201738]
WOS Research Area
Geology
WOS Subject
Geosciences, Multidisciplinary
WOS Accession No
WOS:000822782100002
Publisher
EI Accession Number
20222512249145
EI Keywords
Biogeochemistry ; Chemical analysis ; Dynamics ; Environmental impact ; Nanotechnology ; Organic compounds ; Scanning electron microscopy ; Shale gas
ESI Classification Code
Environmental Impact and Protection:454.2 ; Geochemistry:481.2 ; Natural Gas Deposits:512.2 ; Gas Fuels:522 ; Nanotechnology:761 ; Biochemistry:801.2 ; Organic Compounds:804.1 ; Physical Properties of Gases, Liquids and Solids:931.2
ESI Research Field
GEOSCIENCES
Data Source
Web of Science
Citation statistics
Cited Times [WOS]:0
Document TypeJournal Article
Identifierhttp://kc.sustech.edu.cn/handle/2SGJ60CL/356193
DepartmentSchool of Environmental Science and Engineering
Affiliation
1.Peking Univ, Coll Engn, BIC ESAT ERE & SKLTCS, Beijing 100871, Peoples R China
2.Southern Univ Sci & Technol, Sch Environm Sci & Engn, Shenzhen 518055, Peoples R China
Corresponding Author AffilicationSchool of Environmental Science and Engineering
Recommended Citation
GB/T 7714
Zhang, Wei,Zhang, Dongxiao,Zhao, Junliang. Experimental study of the influence of geochemical features on the viscoelasticity of organic matter in shale[J]. MARINE AND PETROLEUM GEOLOGY,2022,143.
APA
Zhang, Wei,Zhang, Dongxiao,&Zhao, Junliang.(2022).Experimental study of the influence of geochemical features on the viscoelasticity of organic matter in shale.MARINE AND PETROLEUM GEOLOGY,143.
MLA
Zhang, Wei,et al."Experimental study of the influence of geochemical features on the viscoelasticity of organic matter in shale".MARINE AND PETROLEUM GEOLOGY 143(2022).
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