Title | Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features |
Author | |
Corresponding Author | Lu,Zhouguang |
Publication Years | 2022-11-01
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DOI | |
Source Title | |
ISSN | 0144-8617
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Volume | 295 |
Abstract | This paper reports a versatile and dynamic hydrogel system based on ultrafast coordination between partially hydrogen-bonded (PHB) biopolymer hyaluronic acid and a series of transition metal ions at appropriate pH values. It was found that the procedure for the hydrogel synthesis was extremely facile, requiring a simple mixing of the components within 2 s. The hydrogels exhibited high water content, up to 96 %. Even so, the hydrogels can be stretched >50 times and rapidly self-heal from damage within only 10 s without using any healing agents or heating. Furthermore, this dynamic hydrogel network underwent reversible sol-gel transitions as response to multiple disparate stimuli, including pH, temperature, ions, redox, and light. The photo-patterning ability of the hydrogel with a rapid gel-sol transition upon exposure to light was also demonstrated. We disclosed the principle and methodology to use PHB metal-biopolymer systems for constructing dynamic bio-related soft matters. |
Keywords | |
URL | [Source Record] |
Indexed By | |
Language | English
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SUSTech Authorship | Corresponding
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Funding Project | National Natural Science Foundation of China[21875097];National Natural Science Foundation of China[21905002];
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EI Accession Number | 20223012400394
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EI Keywords | Biomolecules
; Biopolymers
; Hyaluronic acid
; Hydrogels
; Hydrogen
; Metal ions
; Organic acids
; Self-healing materials
; Sol-gels
; Transition metal compounds
; Transition metals
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ESI Classification Code | Metals, Plastics, Wood and Other Structural Materials:415
; Biological Materials and Tissue Engineering:461.2
; Biology:461.9
; Metallurgy and Metallography:531
; Metallurgy:531.1
; Biochemistry:801.2
; Colloid Chemistry:801.3
; Physical Chemistry:801.4
; Chemical Products Generally:804
; Organic Compounds:804.1
; Polymeric Materials:815.1
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ESI Research Field | CHEMISTRY
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Scopus EID | 2-s2.0-85134492397
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Data Source | Scopus
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Citation statistics |
Cited Times [WOS]:4
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Document Type | Journal Article |
Identifier | http://kc.sustech.edu.cn/handle/2SGJ60CL/359513 |
Department | Department of Materials Science and Engineering |
Affiliation | 1.School of Chemistry and Chemical Engineering,Anyang Normal University,Anyang,Anyang,455000,China 2.Department of Materials Science and Engineering,Shenzhen Key Laboratory of Interfacial Science and Engineering of Materials,Southern University of Science and Technology,Shenzhen,518055,China |
Corresponding Author Affilication | Department of Materials Science and Engineering |
Recommended Citation GB/T 7714 |
Sun,Zhifang,Lyu,Fucong,Wu,Shaofei,et al. Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features[J]. CARBOHYDRATE POLYMERS,2022,295.
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APA |
Sun,Zhifang,Lyu,Fucong,Wu,Shaofei,Lu,Zhouguang,&Cheng,Hua.(2022).Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features.CARBOHYDRATE POLYMERS,295.
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MLA |
Sun,Zhifang,et al."Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features".CARBOHYDRATE POLYMERS 295(2022).
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