中文版 | English
Title

Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features

Author
Corresponding AuthorLu,Zhouguang
Publication Years
2022-11-01
DOI
Source Title
ISSN
0144-8617
Volume295
Abstract
This paper reports a versatile and dynamic hydrogel system based on ultrafast coordination between partially hydrogen-bonded (PHB) biopolymer hyaluronic acid and a series of transition metal ions at appropriate pH values. It was found that the procedure for the hydrogel synthesis was extremely facile, requiring a simple mixing of the components within 2 s. The hydrogels exhibited high water content, up to 96 %. Even so, the hydrogels can be stretched >50 times and rapidly self-heal from damage within only 10 s without using any healing agents or heating. Furthermore, this dynamic hydrogel network underwent reversible sol-gel transitions as response to multiple disparate stimuli, including pH, temperature, ions, redox, and light. The photo-patterning ability of the hydrogel with a rapid gel-sol transition upon exposure to light was also demonstrated. We disclosed the principle and methodology to use PHB metal-biopolymer systems for constructing dynamic bio-related soft matters.
Keywords
URL[Source Record]
Indexed By
Language
English
SUSTech Authorship
Corresponding
Funding Project
National Natural Science Foundation of China[21875097];National Natural Science Foundation of China[21905002];
EI Accession Number
20223012400394
EI Keywords
Biomolecules ; Biopolymers ; Hyaluronic acid ; Hydrogels ; Hydrogen ; Metal ions ; Organic acids ; Self-healing materials ; Sol-gels ; Transition metal compounds ; Transition metals
ESI Classification Code
Metals, Plastics, Wood and Other Structural Materials:415 ; Biological Materials and Tissue Engineering:461.2 ; Biology:461.9 ; Metallurgy and Metallography:531 ; Metallurgy:531.1 ; Biochemistry:801.2 ; Colloid Chemistry:801.3 ; Physical Chemistry:801.4 ; Chemical Products Generally:804 ; Organic Compounds:804.1 ; Polymeric Materials:815.1
ESI Research Field
CHEMISTRY
Scopus EID
2-s2.0-85134492397
Data Source
Scopus
Citation statistics
Cited Times [WOS]:4
Document TypeJournal Article
Identifierhttp://kc.sustech.edu.cn/handle/2SGJ60CL/359513
DepartmentDepartment of Materials Science and Engineering
Affiliation
1.School of Chemistry and Chemical Engineering,Anyang Normal University,Anyang,Anyang,455000,China
2.Department of Materials Science and Engineering,Shenzhen Key Laboratory of Interfacial Science and Engineering of Materials,Southern University of Science and Technology,Shenzhen,518055,China
Corresponding Author AffilicationDepartment of Materials Science and Engineering
Recommended Citation
GB/T 7714
Sun,Zhifang,Lyu,Fucong,Wu,Shaofei,et al. Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features[J]. CARBOHYDRATE POLYMERS,2022,295.
APA
Sun,Zhifang,Lyu,Fucong,Wu,Shaofei,Lu,Zhouguang,&Cheng,Hua.(2022).Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features.CARBOHYDRATE POLYMERS,295.
MLA
Sun,Zhifang,et al."Ultrafast construction of partially hydrogen-bonded metal-hyaluronan networks with multiple biotissue-related features".CARBOHYDRATE POLYMERS 295(2022).
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Export to Excel
Export to Csv
Altmetrics Score
Google Scholar
Similar articles in Google Scholar
[Sun,Zhifang]'s Articles
[Lyu,Fucong]'s Articles
[Wu,Shaofei]'s Articles
Baidu Scholar
Similar articles in Baidu Scholar
[Sun,Zhifang]'s Articles
[Lyu,Fucong]'s Articles
[Wu,Shaofei]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Sun,Zhifang]'s Articles
[Lyu,Fucong]'s Articles
[Wu,Shaofei]'s Articles
Terms of Use
No data!
Social Bookmark/Share
No comment.

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.