Controllable Synthesis of 2D Materials by Electrochemical Exfoliation for Energy Storage and Conversion Application

Lu, Xueyi1; Cai, Mohang1; Wu, Xuemin1; Zhang, Yongfei1; Li, Shuai2,3; Liao, Shijun4; Lu, Xia1

2022-12-01

10.1002/smll.202206702

Small   Impact Factor & Quartile

1613-6810

1613-6829

2D materials have captured much recent research interest in a broad range of areas, including electronics, biology, sensors, energy storage, and others. In particular, preparing 2D nanosheets with high quality and high yield is crucial for the important applications in energy storage and conversion. Compared with other prevailing synthetic strategies, the electrochemical exfoliation of layered starting materials is regarded as one of the most promising and convenient methods for the large-scale production of uniform 2D nanosheets. Here, recent developments in electrochemical delamination are reviewed, including protocols, categories, principles, and operating conditions. State-of-the-art methods for obtaining 2D materials with small numbers of layers-including graphene, black phosphorene, transition metal dichalcogenides and MXene-are also summarized and discussed in detail. The applications of electrochemically exfoliated 2D materials in energy storage and conversion are systematically reviewed. Drawing upon current progress, perspectives on emerging trends, existing challenges, and future research directions of electrochemical delamination are also offered.

2D materials anion cations electrochemical exfoliation nanosheets

SCI

English

Corresponding

National Natural Science Foundation of China["22209213","22075328"] ; National Key Research and Development Program of China[2019YFA0705702] ; Natural Science Foundation of Guangdong Province[2022A1515010405] ; Fundamental Research Funds for the Central Universities, Sun Yat-sen University[22qntd0204] ; Guangdong Provincial Key Laboratory of Energy Materials for Electric Power[2018B030322001]

Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics

Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter

WOS:000897946400001

WILEY-V C H VERLAG GMBH

Web of Science

1.Sun Yat Sen Univ, Sch Mat, Shenzhen 518107, Peoples R China
2.Southern Univ Sci & Technol, Dept Phys, Guangdong Prov Key Lab Energy Mat Elect Power, Shenzhen 518055, Peoples R China
3.Southern Univ Sci & Technol, Acad Adv Interdisciplinary Studies, Shenzhen 518055, Peoples R China
4.Southern Univ Sci & Technol, Acad Adv Interdisciplinary Studies, Shenzhen 518055, Peoples R China

Lu, Xueyi,Cai, Mohang,Wu, Xuemin,et al. Controllable Synthesis of 2D Materials by Electrochemical Exfoliation for Energy Storage and Conversion Application[J]. Small,2022.

Lu, Xueyi.,Cai, Mohang.,Wu, Xuemin.,Zhang, Yongfei.,Li, Shuai.,...&Lu, Xia.(2022).Controllable Synthesis of 2D Materials by Electrochemical Exfoliation for Energy Storage and Conversion Application.Small.

Lu, Xueyi,et al."Controllable Synthesis of 2D Materials by Electrochemical Exfoliation for Energy Storage and Conversion Application".Small (2022).