中文版 | English
Title

Differentiated Ionic Electroresponse of Asymmetric Bio-Hydrogels with Unremitting Power Output

Author
Corresponding AuthorHe, Jiaqing; Ho, Ghim Wei
Publication Years
2023-02-01
DOI
Source Title
ISSN
1614-6832
EISSN
1614-6840
Abstract
Cytomembranes with efficient ionic selectivity and energy circulation, essential for biological activities in multicellular organisms, are a source of inspiration for man-made biomedical devices. However, current man-made soft systems mainly imitate simple and passive cytomembranes behaviors, restrained by the grand challenge that lies at the meeting point of synchronous engineering of both (dynamic) ionic selectivity and (passive) transcellular-like potential in one structure. Here a dynamically differentiated ionic electroresponse and passive incessant power output of an asymmetric bio-hydrogel constructed using a simple self-propagative flow approach are reported. The unprecedented freely formed p and n analogue hydrogels yield a transcellular-like potential (110-200 mV) in response to diverse stimuli-where the cathode or anode is capable of perceivable electroresponse to water and/or salt media, respectively. A single hydrogel can generate an output power density of 135-190 mW m(-2) superior to most bio-inspired soft and/or green power sources. The scalable manufacturing and proof-of-concept demonstration elucidate the feasibility of mobilizing passive and dynamic behaviors in one structure. This work has the potential for realizing high-performance soft power sources in parallel to electrostimulation for neural excitation/inhibition, extending into the previously inaccessible region of biomedical applications.
Keywords
URL[Source Record]
Indexed By
Language
English
SUSTech Authorship
Corresponding
Funding Project
A*STAR["2019 AME IRG","A2083c0059"] ; National University of Singapore[A-0005947-24-00]
WOS Research Area
Chemistry ; Energy & Fuels ; Materials Science ; Physics
WOS Subject
Chemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
WOS Accession No
WOS:000930013200001
Publisher
Data Source
Web of Science
Citation statistics
Cited Times [WOS]:0
Document TypeJournal Article
Identifierhttp://kc.sustech.edu.cn/handle/2SGJ60CL/479599
DepartmentDepartment of Physics
Affiliation
1.Natl Univ Singapore, Dept Elect & Comp Engn, 4 Engn Dr 3, Singapore 117583, Singapore
2.Univ Elect Sci & Technol China, Sch Phys, Chengdu 611731, Peoples R China
3.Southern Univ Sci & Technol, Dept Phys, Shenzhen 518055, Peoples R China
4.Natl Univ Singapore, Dept Mat Sci & Engn, 9 Engn Dr 1, Singapore 117575, Singapore
Corresponding Author AffilicationDepartment of Physics
Recommended Citation
GB/T 7714
Pan, Xinglong,Jin, Yakang,Zhou, Yi,et al. Differentiated Ionic Electroresponse of Asymmetric Bio-Hydrogels with Unremitting Power Output[J]. Advanced Energy Materials,2023.
APA
Pan, Xinglong.,Jin, Yakang.,Zhou, Yi.,Wang, Xiao-Qiao.,Lu, Wanheng.,...&Ho, Ghim Wei.(2023).Differentiated Ionic Electroresponse of Asymmetric Bio-Hydrogels with Unremitting Power Output.Advanced Energy Materials.
MLA
Pan, Xinglong,et al."Differentiated Ionic Electroresponse of Asymmetric Bio-Hydrogels with Unremitting Power Output".Advanced Energy Materials (2023).
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