| Title | Review on Electrochemical Reduction of Nitrogen by Graphdiyne- Based Catalysts: Recent Advances and Outlook |
| Author | |
| Corresponding Author | Duan, Lele |
| Publication Years | 2023-02-01
|
| DOI | |
| Source Title | |
| ISSN | 0887-0624
|
| EISSN | 1520-5029
|
| Abstract | The present industrial ammonia synthesis is overdependent on the Haber-Bosch process operating under harsh conditions, which consumes enormous global energy together with gigatons of greenhouse gas emissions annually. The electrochemical nitrogen reduction reaction (NRR) offers a green and sustainable approach to ammonia synthesis under mild reaction conditions while its efficiency has been plagued by sluggish reactivity. Recently, novel engineering of catalysts and the development of electrolyzers have highlighted compelling opportunities to optimize the performance of the electrochemical NRR. In this review, emphasis was paid to summarizing a novel family of graphdiyne-based nitrogen reduction electrocatalysts together with a brief introduction to the fundamentals of the electrochemical NRR. In the beginning, mechanisms of the electrochemical NRR are discussed, followed by the elucidation of different types of electrolyzers together with experimental aspects of catalyst evaluation. Then, the advances in graphdiyne-based electrocatalysts are highlighted. Finally, the critical challenges and outlook for the emerging paradigms in the rational design of nitrogen reduction electrocatalysts are proposed. |
| URL | [Source Record] |
| Indexed By | |
| Language | English
|
| SUSTech Authorship | First
; Corresponding
|
| Funding Project | National Natural Science Foundation of China[22179057]
; Stable Support Plan Program of Shenzhen Natural Science Fund[20200925152742003]
; Educational Commission of Guangdong Province[2020KTSCX121]
|
| WOS Research Area | Energy & Fuels
; Engineering
|
| WOS Subject | Energy & Fuels
; Engineering, Chemical
|
| WOS Accession No | WOS:000934942400001
|
| Publisher | |
| ESI Research Field | ENGINEERING
|
| Data Source | Web of Science
|
| Citation statistics |
Cited Times [WOS]:0
|
| Document Type | Journal Article |
| Identifier | http://kc.sustech.edu.cn/handle/2SGJ60CL/501470 |
| Department | Department of Chemistry 深圳格拉布斯研究院 |
| Affiliation | 1.Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Peoples R China 2.Southern Univ Sci & Technol, Shenzhen Grubbs Inst, Shenzhen 518055, Peoples R China |
| First Author Affilication | Department of Chemistry; Shenzhen Grubbs Institute |
| Corresponding Author Affilication | Department of Chemistry; Shenzhen Grubbs Institute |
| First Author's First Affilication | Department of Chemistry |
| Recommended Citation GB/T 7714 |
Hu, Junhui,Zou, Haiyuan,Li, Fan,et al. Review on Electrochemical Reduction of Nitrogen by Graphdiyne- Based Catalysts: Recent Advances and Outlook[J]. ENERGY & FUELS,2023.
|
| APA |
Hu, Junhui.,Zou, Haiyuan.,Li, Fan.,Wei, Shuting.,Cheng, Minglun.,...&Duan, Lele.(2023).Review on Electrochemical Reduction of Nitrogen by Graphdiyne- Based Catalysts: Recent Advances and Outlook.ENERGY & FUELS.
|
| MLA |
Hu, Junhui,et al."Review on Electrochemical Reduction of Nitrogen by Graphdiyne- Based Catalysts: Recent Advances and Outlook".ENERGY & FUELS (2023).
|
| Files in This Item: | There are no files associated with this item. | |||||
Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.
Edit Comment