中文版 | English
Title

Identifying the dominant carrier of CdSe-based blue quantum dot light-emitting diode

Author
Corresponding AuthorSun, Xiao Wei
Publication Years
2023-03-13
DOI
Source Title
ISSN
0003-6951
EISSN
1077-3118
Volume122Issue:11
Abstract
Unlike red and green quantum dot light-emitting diodes (QLEDs), it is not clear whether a blue QLED is an electron-dominated device. In this work, we identify that electron is over-injected in blue QLEDs by impedance spectroscopy. By analyzing the capacitance-voltage characteristics of the single-carrier devices, we find that the built-in voltage of the electron-only device is smaller than that of the hole-only device. Therefore, electron injection is more efficient than hole injection in blue QLEDs. To support our arguments, we employ a red QD as a fluorescent sensor to spatially investigate the exciton recombination zone of a blue QLED. Consequently, we observe that the exciton recombination zone of the blue QLED is close to the hole transport layer, and it shifts toward an electron transport layer with the increase in the applied bias. Our work provides a practical method for identifying the excess carrier in blue QLEDs, and it could be applied to other types of QLEDs.
URL[Source Record]
Indexed By
Language
English
SUSTech Authorship
First ; Corresponding
Funding Project
National Key Research and Development Program of China["2021YFB3602703","2022YFB3606504","2022YFB3602903"] ; National Natural Science Foundation of China[62122034] ; Guangdong University Key Laboratory for Advanced Quantum Dot Displays[2017KSYS007] ; Shenzhen Key Laboratory for Advanced Quantum Dot Displays and Lighting[ZDSYS201707281632549]
WOS Research Area
Physics
WOS Subject
Physics, Applied
WOS Accession No
WOS:000948796400001
Publisher
ESI Research Field
PHYSICS
Data Source
Web of Science
Citation statistics
Cited Times [WOS]:0
Document TypeJournal Article
Identifierhttp://kc.sustech.edu.cn/handle/2SGJ60CL/523897
DepartmentDepartment of Electrical and Electronic Engineering
Affiliation
1.Southern Univ Sci & Technol, Inst Nanosci & Applicat, Dept Elect & Elect Engn, Shenzhen 518055, Peoples R China
2.Southern Univ Sci & Technol, Hong Kong, Guangdong, Peoples R China
First Author AffilicationDepartment of Electrical and Electronic Engineering;  Southern University of Science and Technology
Corresponding Author AffilicationDepartment of Electrical and Electronic Engineering;  Southern University of Science and Technology
First Author's First AffilicationDepartment of Electrical and Electronic Engineering
Recommended Citation
GB/T 7714
Qu, Xiangwei,Xiang, Guohong,Ma, Jingrui,et al. Identifying the dominant carrier of CdSe-based blue quantum dot light-emitting diode[J]. APPLIED PHYSICS LETTERS,2023,122(11).
APA
Qu, Xiangwei.,Xiang, Guohong.,Ma, Jingrui.,Liu, Pai.,Kyaw, Aung Ko Ko.,...&Sun, Xiao Wei.(2023).Identifying the dominant carrier of CdSe-based blue quantum dot light-emitting diode.APPLIED PHYSICS LETTERS,122(11).
MLA
Qu, Xiangwei,et al."Identifying the dominant carrier of CdSe-based blue quantum dot light-emitting diode".APPLIED PHYSICS LETTERS 122.11(2023).
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