中文版 | English
Title

Dissolvable templates to prepare Pt-based porous metallic glass for the oxygen reduction reaction

Author
Corresponding AuthorRuan, Wenqing; Ma, Jiang
Publication Years
2023-03-01
DOI
Source Title
ISSN
2040-3364
EISSN
2040-3372
Abstract
Oxygen reduction reaction (ORR) plays a crucial role in electrochemical energy conversion and storage devices such as metal-air batteries and water electrolyzers. Herein, a hierarchical nanoporous platinum-based metallic glass (NPMG) was developed by a facile fabrication method by dissolving in a liquid. The surface topography of the sample can be easily modulated by controlling the particle size of sodium chloride. As a result, the NPMG was proved to be efficient and robust as the ORR catalysts with super hydrophilicity and self-renewal capacity. The half-wave potential of the platinum-based porous material was 835 mV at 0.1 M KOH, even higher than that of the commercial Pt/C catalyst (823 mV) and the previously reported platinum material. In particular, platinum-based porous materials have extremely long stability (more than 500 h) through the self-renewal surface, which perfectly meets the requirements of catalyst stability in batteries. Our study has a better inspiration for developing and applying novel catalysts to prepare metal-air batteries.
URL[Source Record]
Indexed By
Language
English
SUSTech Authorship
Others
Funding Project
Key Basic and Applied Research Program of Guangdong Province, China[2019B030302010] ; NSF of China["52122105","52271150","51971150","52201185"] ; National Key Research and Development Program of China[2018YFA0703604]
WOS Research Area
Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS Subject
Chemistry, Multidisciplinary ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied
WOS Accession No
WOS:000955047400001
Publisher
Data Source
Web of Science
Citation statistics
Cited Times [WOS]:0
Document TypeJournal Article
Identifierhttp://kc.sustech.edu.cn/handle/2SGJ60CL/523946
DepartmentDepartment of Mechanics and Aerospace Engineering
Affiliation
1.Shenzhen Univ, Coll Mechatron & Control Engn, Shenzhen Key Lab High Performance Nontradit Mfg, Shenzhen 518060, Peoples R China
2.Southern Univ Sci & Technol, Dept Mech & Aerosp Engn, Shenzhen 518055, Peoples R China
3.Hong Kong Univ Sci & Technol, Dept Mech & Aerosp Engn, Kowloon, Clear Water Bay, Hong Kong, Peoples R China
4.Wuhan Univ Technol, Sch Mat Sci & Engn, Wuhan, Peoples R China
Recommended Citation
GB/T 7714
Liang, Xiong,Liu, Zehang,Fu, Jianan,et al. Dissolvable templates to prepare Pt-based porous metallic glass for the oxygen reduction reaction[J]. NANOSCALE,2023.
APA
Liang, Xiong.,Liu, Zehang.,Fu, Jianan.,Zhang, Heting.,Huang, Jinbiao.,...&Ma, Jiang.(2023).Dissolvable templates to prepare Pt-based porous metallic glass for the oxygen reduction reaction.NANOSCALE.
MLA
Liang, Xiong,et al."Dissolvable templates to prepare Pt-based porous metallic glass for the oxygen reduction reaction".NANOSCALE (2023).
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