中文版 | English
Title

Advances and challenges in single-site catalysts towards electrochemical CO2 methanation

Author
Corresponding AuthorChen, Shenghua; Wang, Dingsheng; Mai, Liqiang
Publication Years
2023-09-01
DOI
Source Title
ISSN
1754-5692
EISSN
1754-5706
Abstract
Electrochemical CO2 reduction to a valuable product is a sustainable and economical method towards carbon neutralization. Among the different products of the electrochemical CO2 reduction reaction (CO2RR), methane is an excellent energy carrier with a high combustion heat. However, for higher methane product selectivity it is crucial to avoid C-C coupling that leads to multi-carbon products. Thus, single-site catalysts (SSCs) with a single active site are ideal candidates. This review summarizes and discusses the current research progress and future application prospects of electrochemical CO2 methanation on SSCs. The CO2 methanation mechanism and primary activity descriptors are discussed in detail with an extensive overview of the coordination structure and design of SSCs, as well as their several in situ characterization methods for tracking the structural changes in SSCs. This review provides insights into the further exploitation of SSCs for selective CO2 methanation that inspires the rational design of SSCs in electrochemical CO2 methanation research.
URL[Source Record]
Indexed By
Language
English
SUSTech Authorship
Others
Funding Project
L. M. acknowledges the National Key Research and Development Program of China (2020YFA0715000), the National Natural Science Foundation of China (51832004, 52127816), and the National Energy-Saving and Low-Carbon Materials Production and Application Demons[2020YFA0715000] ; National Key Research and Development Program of China["51832004","52127816"] ; National Natural Science Foundation of China[TC220H06N] ; National Energy-Saving and Low-Carbon Materials Production and Application Demonstration Platform Program[71211223010707]
WOS Research Area
Chemistry ; Energy & Fuels ; Engineering ; Environmental Sciences & Ecology
WOS Subject
Chemistry, Multidisciplinary ; Energy & Fuels ; Engineering, Chemical ; Environmental Sciences
WOS Accession No
WOS:001075167900001
Publisher
Data Source
Web of Science
Citation statistics
Cited Times [WOS]:0
Document TypeJournal Article
Identifierhttp://kc.sustech.edu.cn/handle/2SGJ60CL/575810
DepartmentDepartment of Mechanical and Energy Engineering
Affiliation
1.Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China
2.UCL, Dept Chem Engn, Electrochem Innovat Lab, London WC1E 7JE, England
3.Xi An Jiao Tong Univ, Sch Chem Engn & Technol, Natl Innovat Platform Ctr Ind Educ Integrat Energy, Xian 710049, Peoples R China
4.Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
5.Southern Univ Sci & Technol, Dept Mech & Energy Engn, Shenzhen 518055, Peoples R China
Recommended Citation
GB/T 7714
Zhu, Jiexin,Lv, Lei,Zaman, Shahid,et al. Advances and challenges in single-site catalysts towards electrochemical CO2 methanation[J]. ENERGY & ENVIRONMENTAL SCIENCE,2023.
APA
Zhu, Jiexin.,Lv, Lei.,Zaman, Shahid.,Chen, Xingbao.,Dai, Yuhang.,...&Mai, Liqiang.(2023).Advances and challenges in single-site catalysts towards electrochemical CO2 methanation.ENERGY & ENVIRONMENTAL SCIENCE.
MLA
Zhu, Jiexin,et al."Advances and challenges in single-site catalysts towards electrochemical CO2 methanation".ENERGY & ENVIRONMENTAL SCIENCE (2023).
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